NaI and TlI are very volatile materials when melted, and crystal growth has a tendency to push impurities back to melt, so it is difficult to make an optimum concentration of Tl(activator) and minimize Tl concentration difference between the top and bottom of a crystal. Conventional crystal growth methods produce a long height and a comparably narrow diameter (Figure I-19 (1)), so the Tl concentration difference between top and bottom is quite large. Our grower can grow short and wide-diameter (Figure I-19 (2)) crystals. This method can reduce concentration difference between top and bottom, so we can get quite uniform scintillation properties with our NaI:Tl crystals grown at CUP. For optimum concentration, we have to exercise the process several times to obtain good growing conditions and reduce growth time.We are testing to grow small NaI crystals with the 2 kg Kyropoulos grower and have so far grown eight NaI crystals. Figure I-20 shows the grown NaI crystals, seven are pure NaI and one is 0.1 mol% Tl doped NaI crystal. There were minor issues like bubbles, a central hole, and contamination issues, but some of them were resolved. We need to improve growing conditions of NaI more. CUP-grown NaI crystals were measured with ICP-MS and results are summarized in Table I-2. KY01-1701 and 1702 were grown with the crystal grade NaI powder (Sigma Aldrich, >5N) and from KY01-1703 to 1804 were grown with the Merck NaI powder (4N). The ICP-MS result of KY01-1701 showed quite severe contaminations from quartz felt, so we no longer use quartz felt. In the rest of grown crystals, there are no observable contaminations. We can observe significantly good reduction of impurities in molybdate crystals for the AMoRE experiment but not for NaI crystals. Therefore, highly purified NaI powders are necessary.We have practiced the technique many times to grow good quality NaI crystals. We expect that we soon can be ready for growing large NaI crystals with the 150 kg grower (KY02). Our goal with the large NaI crystal grower is to grow 115 kg of crystals with dimensions of Φ400 mm × 250 mm.